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On Linux:

Compile MCsquare with the command: make
(this should generate the executable MCsquare_linux)

Configure the simulation in config.txt
Then, run MCsquare with the launcher: ./MCsquare


On Windows:

Compile MCsquare by running Makefile.bat
(You may need to adapt the path to librarary directories in Makefile.bat)

Configure the simulation in config.txt
Then, run MCsquare with the launcher: MCsquare.bat